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篇目详细内容 |
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【篇名】 |
Effect of modeling factors on the dissolution-diffusion-convection process during CO2 geological storage in deep saline formations |
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【刊名】 |
Frontiers of Earth Science |
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【刊名缩写】 |
Front. Earth Sci |
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【ISSN】 |
2095-0195 |
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【EISSN】 |
2095-0209 |
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【DOI】 |
10.1007/s11707-013-0359-x |
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【出版社】 |
Higher Education Press and Springer-Verlag Berlin
Heidelberg |
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【出版年】 |
2013 |
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【卷期】 |
7
卷2期 |
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【页码】 |
238-256
页,共
19
页 |
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【作者】 |
Wei ZHANG;
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【关键词】 |
climate change; carbon dioxide; geologic sequestration; density-driven convection; reactive transport modeling; grid resolution |
【摘要】 |
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It is well known that during CO2 geological storage, density-driven convective activity can significantly accelerate the dissolution of injected CO2 into water. This action could limit the escape of supercritical CO2 from the storage formation through vertical pathways such as fractures, faults and abandoned wells, consequently increasing permanence and security of storage. First, we investigated the effect of numerical perturbation caused by time and grid resolution and the convergence criteria on the dissolution-diffusion-convection (DDC) process. Then, using the model with appropriate spatial and temporal resolution, some uncertainty parameters investigated in our previous paper such as initial gas saturation and model boundaries, and other factors such as relative liquid permeability and porosity modification were used to examine their effects on the DDC process. Finally, we compared the effect of 2D and 3D models on the simulation of the DDC process. The above modeling results should contribute to clear understanding and accurate simulation of the DDC process, especially the onset of convective activity, and the CO2 dissolution rate during the convection-dominated stage. |
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